durusmail: mems-talk: Thermal growth rates of Aluminum Oxide
Thermal growth rates of Aluminum Oxide
Thermal growth rates of Aluminum Oxide
RobDavis
2002-06-18
My background is in Materials....

If your problem is related to erosion (mechanical) and less on corrosion
(electrochemical) then one of principal means to combat erosion is to focus
on the strength or hardness (nearly the same).  Ok, now one of most obvious
parameters is the temperature.  The tensile strength of aluminum will change
100 times between 350C and RT and the cryogenic properties of aluminum are
very good..... So the rule would be to consider your process and try to do
everything you can do to keep the temperature down, chill plate, pulse the
ion gun, or stage the process with intermediate cool down steps.  Maintain
good thermal control to maintain high hardness and erosion resistance for
long life.

The second consideration for a strength increase is to alloy it
(metallurgists just love this stuff).  The tensile strength of high purity
fully annealed aluminum is about 1.5 ksi...where as commercial high strength
aluminum can exceed 80-100 ksi.  Alloying additions of one to several
percent can produce significant effects to the mechanical strength.
Realizing we are talking about a sputter deposit material, common sputter
materials like Cr and Cu have limited solubility in aluminum but can change
the strength to an "engineering" value.  One to two weight percent could
make a major difference.  Other "contaminants" like Si, Zn, Mn and Mg also
can be used.  The difference in the atomic radii D=(rx -ral)% can be used to
judge the effect of solid solution strengthening of high purity aluminum.
The D for Si -3.8; Zn -6.0; Cu -10.7; Mn -11.3 and Mg is +11.8.  These
produce a relative increase in tensile strength per wt% of alloy addition of
5.7, 2.2, 6.3, 7.8 and 7.3 respectively.  Therefore a process that adds 2
wt% Cu will change the strength nearly 15%.

Less practical approaches to aluminum strengthening are grain refinement,
precipitation hardening and cold work....like I said less practicable.

I have sputtered using contaminated targets and ended up with several %
contaminant levels in the deposit.

Good luck and let us know how your experiments turn out...MEMS tribology is
an interest to me.
Rob


-----Original Message-----
From: mems-talk-admin@memsnet.org [mailto:mems-talk-admin@memsnet.org]On
Behalf Of Nicholas Jankowski
Sent: Monday, June 17, 2002 9:09 PM
To: mems-talk@memsnet.org
Subject: [mems-talk] Thermal growth rates of Aluminum Oxide


New to the list.  I searched through the archives and didn't find this
question, but if its there and anyone can point me to the thread I'd be
obliged.  Anyway, here we go:

Performing some relatively deep RIE of SiO2 using an aluminum mask.
Problem is that mask is eroding more than we'd like (it's not
sacrificial), even after trying to tweak the recipe.  What we are
looking at now are ways to 'harden' this aluminum mask such that the
unwanted milling will be reduced.  The mask is only 15m thick (not
negotiable), and we need the majority of the mask to remain aluminum for
functionality after processing.  What we had in mind was enhancing the
oxidation of the aluminum, making for a thicker Al2O3 layer at the top
of the metal than the normal native oxide.  Even though it is likely to
still be milled away, the thicker oxide should last longer and result in
less overall aluminum milling.  Not sure on thickness requirements, as I
don't quite know the etch selectivity between Al2O3 and Al, but the
normal process is currently milling away about 30-40% of the thickness,
so we'd probably want to find the optimum somewhere between the native
2.5nm and 250nm.

Here's the problem:  I've been hunting through the literature trying to
find something for Aluminum like the SiO2 oxidation curves that I could
find in 5 minutes if I needed to.  Basically, I need to know aluminum
oxide thickness as a function of time _at elevated temperatures_, and so
far I've been coming up short.  Would anyone out there be able to point
me to the appropriate reference, or at least in the right direction?

Also, I've seen that plasma oxidation could be another option instead of
thermal oxidation, and possibly a better one since it wouldn't require
temperatures as high, and we could keep the wafer in the closed system
for both processes.  Any advice on this would be greatly appreciated as
well.

If providing more info would be helpful, I'd be happy to do so.  Thanks.
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